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A new feature lets you set an alarm to remind you when new pages are added to the site.. will not be published or shared.Highly Selective Nitroxide Radical Generation at the Nanoscale and the Importance of the Cation-Anion Distance.
Understanding the chemical mechanisms of the generation of nitroxide radicals at the surface of small, highly dispersed, metal oxide nanoparticles is a topic of great interest. A number of radicalizing reactions have been reported for the cationic-anionic redox cycle (RKC reaction) that includes oxidative addition and reduction of the surface metal oxide. However, it has been established that the RKC reaction does not explain the observed accumulation of nitroxide radicals on the surface of a few metal oxides. The present work shows that neither the initial nucleophilic attack of the water molecules on the oxide nor the fast reduction of hydroxyl radical to water nor the common cation-anion reactions that are involved in the RKC reaction are involved in the nitroxide radical generation in the gas phase. The results demonstrate a clear distinction between the anion-cation reactions, which are involved in the RKC reaction, and the cation-anion reactions, which leads to the formation of the nitroxide radical. In particular, the cation-anion reactions are found to induce the formation of N-O bonds in the nitroxide radical through a rearrangement process, which is not available through the RKC reaction.The ever-expanding smartphone market has transformed the landscape of home theater gear. Some people, however, still harbor the need for a high-def TV that doesn’t require them to wade through dozens of cables.
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